Observational evidence for aerosols increasing upper tropospheric humidity

Laura Riuttanen, Marja Bister, Veli-Matti Kerminen, Viju O. John, Anu-Maija Sundstrom, Miikka Dal Maso, Jouni Räisänen, Victoria A. Sinclair, Risto Makkonen, Filippo Xausa, Gerrit de Leeuw, Markku Kulmala

    Research output: Contribution to journalArticleScientificpeer-review

    8 Citations (Scopus)
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    Abstract

    Aerosol-cloud interactions are the largest source of uncertainty in the radiative forcing of the global climate. A phenomenon not included in the estimates of the total net forcing is the potential increase in upper tropospheric humidity (UTH) by anthropogenic aerosols via changes in the microphysics of deep convection. Using remote sensing data over the ocean east of China in summer, we show that increased aerosol loads are associated with an UTH increase of 2.2 +/- 1.5 in units of relative humidity. We show that humidification of aerosols or other meteorological covariation is very unlikely to be the cause of this result, indicating relevance for the global climate. In tropical moist air such an UTH increase leads to a regional radiative effect of 0.5 +/- 0.4 W m(-2). We conclude that the effect of aerosols on UTH should be included in future studies of anthropogenic climate change and climate sensitivity.

    Original languageEnglish
    Pages (from-to)14331-14342
    Number of pages12
    JournalAtmospheric Chemistry and Physics
    Volume16
    Issue number22
    DOIs
    Publication statusPublished - 17 Nov 2016
    Publication typeA1 Journal article-refereed

    Keywords

    • DEEP CONVECTIVE CLOUDS
    • GENERAL-CIRCULATION MODEL
    • RADIATIVE-TRANSFER
    • OPTICAL DEPTH
    • REANALYSIS
    • SATELLITE
    • ALGORITHM
    • CLIMATE
    • SYSTEM

    Publication forum classification

    • Publication forum level 3

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