An Epsilon-Near-Zero-Based Nonlinear Platform for Ultrafast Re-Writable Holography

We re-examine real-time holography for all-optical structuring of light and optical computation using a contemporary material: a subwavelength-thick, spatially unstructured film of indium tin oxide (ITO). When excited by spatially structured light at epsilon-near-zero frequencies, the film acts as an efficient and reconfigurable diffractive optical platform for all-optical modulation of light such as spatial structuring and optical computations. We demonstrate a few percent of absolute diffraction efficiency over greater than 300-nm-bandwidth around telecom wavelengths using a film four orders of magnitude thinner than and up to six orders of magnitude faster than standard holographic materials. Our findings highlight the potential of using epsilon-near-zero-based nanostructures for efficient modulation of spatially structured light and rapid prototyping without complex nanofabrication processes.