Dipole limit in second-harmonic generation from arrays of gold nanoparticles

Robert Czaplicki; Mariusz Zdanowicz; Kalle Koskinen; Janne Lakkanen; Markku Kuittinen; Martti Kauranen

doi:10.1364/OE.19.026866

Dipole limit in second-harmonic generation from arrays of gold nanoparticles

Julkaisun otsikon käännös: Dipole limit in second-harmonic generation from arrays of gold nanoparticles

Robert Czaplicki
, Mariusz Zdanowicz
, Kalle Koskinen
, Janne Lakkanen
, Markku Kuittinen
, Martti Kauranen

Tutkimustuotos: Artikkeli › Tieteellinen › vertaisarvioitu

69 Sitaatiot (Scopus)

26 Lataukset (Pure)

Abstrakti

We present a multipolar tensor analysis of second-harmonic generation from arrays of noncentrosymmetric gold nanoparticles. In contrast to earlier results, where higher multipoles and symmetry-forbidden signals arising from sample defects play a significant role, the present results are completely dominated by symmetry-allowed electric-dipole tensor components. The result arises from significant improvement in sample quality, which suppresses the higher-multipole effects and enhances the overall response by an order of magnitude. The results are a prerequisite for metamaterials with controllable nonlinear properties.

Julkaisun otsikon käännös	Dipole limit in second-harmonic generation from arrays of gold nanoparticles
Alkuperäiskieli	Englanti
Sivut	26866-26870
Julkaisu	Optics Express
Vuosikerta	19
Numero	27
DOI - pysyväislinkit	https://doi.org/10.1364/OE.19.026866
Tila	Julkaistu - 2011
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Julkaisufoorumi-taso

Jufo-taso 2

Pääsy asiakirjaan

10.1364/OE.19.026866

Czaplicki dipole limit in second-harmonic generation
This paper was published in Optics Express and is made available as an electronic reprint with the permission of OSA. The paper can be found at the following URL on the OSA website: http://www.opticsinfobase.org/oe/abstract.cfm?uri=oe-19-27-26866. Systematic or multiple reproduction or distribution to multiple locations via electronic or other means is prohibited and is subject to penalties under law.

http://urn.fi/URN:NBN:fi:tty-201210191320

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author = "Robert Czaplicki and Mariusz Zdanowicz and Kalle Koskinen and Janne Lakkanen and Markku Kuittinen and Martti Kauranen",

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T1 - Dipole limit in second-harmonic generation from arrays of gold nanoparticles

AU - Czaplicki, Robert

AU - Zdanowicz, Mariusz

AU - Koskinen, Kalle

AU - Lakkanen, Janne

AU - Kuittinen, Markku

AU - Kauranen, Martti

N1 - Poistettu tupla r=1829<br/>Contribution: organisation=fys,FACT1=1<br/>Publisher name: Optical Society of America - OSA

PY - 2011

Y1 - 2011

N2 - We present a multipolar tensor analysis of second-harmonic generation from arrays of noncentrosymmetric gold nanoparticles. In contrast to earlier results, where higher multipoles and symmetry-forbidden signals arising from sample defects play a significant role, the present results are completely dominated by symmetry-allowed electric-dipole tensor components. The result arises from significant improvement in sample quality, which suppresses the higher-multipole effects and enhances the overall response by an order of magnitude. The results are a prerequisite for metamaterials with controllable nonlinear properties.

AB - We present a multipolar tensor analysis of second-harmonic generation from arrays of noncentrosymmetric gold nanoparticles. In contrast to earlier results, where higher multipoles and symmetry-forbidden signals arising from sample defects play a significant role, the present results are completely dominated by symmetry-allowed electric-dipole tensor components. The result arises from significant improvement in sample quality, which suppresses the higher-multipole effects and enhances the overall response by an order of magnitude. The results are a prerequisite for metamaterials with controllable nonlinear properties.

U2 - 10.1364/OE.19.026866

DO - 10.1364/OE.19.026866

M3 - Article

SN - 1094-4087

VL - 19

SP - 26866

EP - 26870

JO - Optics Express

JF - Optics Express

IS - 27

ER -

Dipole limit in second-harmonic generation from arrays of gold nanoparticles

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