Nonlinear optical activity effects in complex anisotropic three-dimensional media

Mikko J. Huttunen; Mari Partanen; Godofredo Bautista; Shi-Wei Chu; Martti Kauranen

doi:10.1364/OME.5.000011

Nonlinear optical activity effects in complex anisotropic three-dimensional media

Mikko J. Huttunen, Mari Partanen, Godofredo Bautista, Shi-Wei Chu, Martti Kauranen

Tutkimustuotos: Artikkeli › Scientific › vertaisarvioitu

6 Sitaatiot (Scopus)

Abstrakti

We perform numerical modelling of nonlinear optical (NLO) microscopy of complex anisotropic three-dimensional (3D) media using the uncoupled dipole approximation. The modelling is applied to 3D biological microstructures resembling collagen fibers and multilamellar vesicles. The results elucidate how nonlinear optical activity effects, such as secondharmonic generation circular dichroism, can arise from 3D morphological chirality, in addition to molecular level chirality. We also show how thirdharmonic generation circular dichroism could act as a contrast mechanism for visualizing local structural ordering in 3D anisotropic materials.

Alkuperäiskieli	Englanti
Sivut	11-21
Sivumäärä	11
Julkaisu	Optical Materials Express
Vuosikerta	5
Numero	1
DOI - pysyväislinkit	https://doi.org/10.1364/OME.5.000011
Tila	Julkaistu - 2015
OKM-julkaisutyyppi	A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Julkaisufoorumi-taso

Jufo-taso 1

!!ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials

Pääsy asiakirjaan

10.1364/OME.5.000011

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title = "Nonlinear optical activity effects in complex anisotropic three-dimensional media",

abstract = "We perform numerical modelling of nonlinear optical (NLO) microscopy of complex anisotropic three-dimensional (3D) media using the uncoupled dipole approximation. The modelling is applied to 3D biological microstructures resembling collagen fibers and multilamellar vesicles. The results elucidate how nonlinear optical activity effects, such as secondharmonic generation circular dichroism, can arise from 3D morphological chirality, in addition to molecular level chirality. We also show how thirdharmonic generation circular dichroism could act as a contrast mechanism for visualizing local structural ordering in 3D anisotropic materials.",

author = "Huttunen, {Mikko J.} and Mari Partanen and Godofredo Bautista and Shi-Wei Chu and Martti Kauranen",

year = "2015",

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T1 - Nonlinear optical activity effects in complex anisotropic three-dimensional media

AU - Huttunen, Mikko J.

AU - Partanen, Mari

AU - Bautista, Godofredo

AU - Chu, Shi-Wei

AU - Kauranen, Martti

PY - 2015

Y1 - 2015

N2 - We perform numerical modelling of nonlinear optical (NLO) microscopy of complex anisotropic three-dimensional (3D) media using the uncoupled dipole approximation. The modelling is applied to 3D biological microstructures resembling collagen fibers and multilamellar vesicles. The results elucidate how nonlinear optical activity effects, such as secondharmonic generation circular dichroism, can arise from 3D morphological chirality, in addition to molecular level chirality. We also show how thirdharmonic generation circular dichroism could act as a contrast mechanism for visualizing local structural ordering in 3D anisotropic materials.

AB - We perform numerical modelling of nonlinear optical (NLO) microscopy of complex anisotropic three-dimensional (3D) media using the uncoupled dipole approximation. The modelling is applied to 3D biological microstructures resembling collagen fibers and multilamellar vesicles. The results elucidate how nonlinear optical activity effects, such as secondharmonic generation circular dichroism, can arise from 3D morphological chirality, in addition to molecular level chirality. We also show how thirdharmonic generation circular dichroism could act as a contrast mechanism for visualizing local structural ordering in 3D anisotropic materials.

UR - http://www.scopus.com/inward/record.url?scp=84920996741&partnerID=8YFLogxK

U2 - 10.1364/OME.5.000011

DO - 10.1364/OME.5.000011

M3 - Article

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VL - 5

SP - 11

EP - 21

JO - Optical Materials Express

JF - Optical Materials Express

SN - 2159-3930

IS - 1

ER -

Nonlinear optical activity effects in complex anisotropic three-dimensional media

Abstrakti

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!!ASJC Scopus subject areas

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